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Various kinds of stimuli-responsiveness have been achieved by incorporating stimuli-sensitive groups into the building blocks in the supramolecular systems, such as pH, light, temperature, redox, and CO 2 responsiveness. Therein, facilely available and tractable pH, light, CO 2 , and enzyme triggers have attracted increasing attention.
Therefore, the morphology and property transformations of self-assembled nanostructures can be modulated effectively and efficiently. The stimuli-triggered morphology transformation of supramolecular assemblies provides a powerful approach to prepare functional organic nanomaterials with well-defined structures in water. Through this approach, nanomaterials with complex and unique morphologies e. The dynamic nature of these in situ supramolecular transformations enables applications in photo-electrical devices, sensing, hierarchical cargo release, and in the construction of metastable materials, etc.
Herein, we review the morphology transformations of self-assembled organic nanomaterials in aqueous solution induced by pH, light, CO 2 , or enzyme-triggered chemical structure changes. This review mainly focuses on the design, transformation conditions, morphology changes, mechanisms, and possible functions of the supramolecular transformation systems. The article was received on 06 Mar , accepted on 21 May and first published on 24 May If you are not the author of this article and you wish to reproduce material from it in a third party non-RSC publication you must formally request permission using Copyright Clearance Center.
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Light Techniques That Trigger Transformation
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